Authors

YUXUAN RUAN

Type

Text

Type

Thesis

Advisor

Dudley, Michael | Koga, Tadanori | Venkatesh, T. A..

Date

2012-05-01

Keywords

Materials Science | clay, dead layer, polystyrene, scCO2, two interfacial effect

Department

Department of Materials Science and Engineering

Language

en_US

Source

This work is sponsored by the Stony Brook University Graduate School in compliance with the requirements for completion of degree.

Identifier

http://hdl.handle.net/11401/71383

Publisher

The Graduate School, Stony Brook University: Stony Brook, NY.

Format

application/pdf

Abstract

A polymer dead layer is a very thin interfacial layer of polymer formed at the solid substrate interface, with no thermal expansion coefficient and molecular mobility. The polymer dead layer has many unique properties compared to the bulk polymer, including the mobility of polymer chains, glass transition temperature, viscosity and so on. In this thesis, organic clay nanoparticles are used as a nanofiller to see how the properties/structures a polystyrene dead layer can be altered. To characterize the structures of PS/clay dead layers, we used ellipsometry, X-ray scattering techniques, and atomic force microscopy (AFM). In addition, supercritical carbon dioxide was used as a screening solvent to control the polymer/substrate interactions. | 29 pages

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