Authors

Jack Lombardi

Type

Text

Type

Dissertation

Advisor

Gersappe, Dilip | Rafailovich, Miriam | Sokolov, Johnathan | Mammone, Thomas.

Date

2014-12-01

Keywords

Clay, Hydrogels, Rheology | Engineering

Department

Department of Materials Science and Engineering.

Language

en_US

Source

This work is sponsored by the Stony Brook University Graduate School in compliance with the requirements for completion of degree.

Identifier

http://hdl.handle.net/11401/76331

Publisher

The Graduate School, Stony Brook University: Stony Brook, NY.

Format

application/pdf

Abstract

Engineered Polymer hydrogels and hydrogels from Bio macromolecules have visco-elastic properties that can be measured using Oscillatory Shear Rheology. Manipulation and measurement of physical properties in gels including F-127 Pluronic Block Co-Polymer and Poly(N-isopropylacrylamide)-Clay are shown through OSR by addition of salts, clays and glucose at physiological levels. Rheological analysis of f-127 illustrates changes in G' reduction with phase transition temperature. Measurements also indicate physical changes due to the aforementioned additives vary as a function of the gel physical and chemical structure. In particular, non-enzymatic glycation is shown to change the modulus of elasticity in both of the gels tested. Rheological analysis is also interpreted to produce a reduction In gel mesh size in the PNIPA -clay gels due to a possible co-solvency between phases of varying degrees of hydration. | 63 pages

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